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Robert Shiller's shocking call: Buy Greek stocks!

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While economist Robert Shiller finds American stocks to be expensive, he suggests that battered Greek equities may actually present a compelling opportunity for savvy investors.

The Nobel prize-winning Yale economist is famous for his valuation-based view of markets. In the long-run, low price-to-earnings ratios provide attractive long-term opportunities, and richly valued markets require caution, his work has shown.

Read MoreThis is Greece's real risk to asset prices: Analyst

Human psychology is what tends to get in the way and to create such opportunities, causing investors to become overly pessimistic at times when stocks are attractive, and far too optimistic in the midst of the bubbles, he has said.

It is perhaps only in the context of his well-known financial and psychological framework that Shiller's latest investment idea can be properly understood.

In an interview Thursday on the CNBC.com program "Trading Nation," Shiller said that stocks in the U.S. are likely to provide only low returns in the medium-term, but "There's also the rest of the world. The U.S. is an expensive market; practically anywhere else is cheaper."

When pressed on where the best value might be found now, Shiller quickly responded: "Greece!"

The economist went on to say that he's not rushing to invest too heavily in Greece. "Maybe I should. I think a little bit in Greece, maybe. One feels fearful, though. I feel fearful about that. It seems awfully edge-of-the-cliff right now, doesn't it?"

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He did not respond to a CNBC email sent Sunday night after Greeks overwhelmingly voted against a new austerity package.

After the vote, JPMorgan's Europe economic research team concluded that "there is now a high likelihood of a Greek exit from the euro, and possibly under chaotic circumstances," although views on this matter are sharply divided.

Greece's Athex Composite Index has fallen 40 percent in the past year, while America's large-cap index is up nearly 5 percent.

That may have created some attractive valuations. For instance, the second-largest stock in that index, Bank of Cyprus, is trading at a forward price-to-earnings valuation of 11, according to FactSet.

Read More Mohamed El-Erian: Grexit 'high probability'

Yet needless to say, the risks inherent in Greek-exposed bank stocks are great. For that reason, Shiller says diversification becomes especially important.

"The secret," he said, "is never to put too much money into investments like that."

Read MoreS&P: 'Grexit' now more likely than not

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